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Metal-Free C-H Amination for Indole Synthesis
- Authors
- Jang, Young Ho; Youn, So Won
- Issue Date
- Jul-2014
- Publisher
- AMER CHEMICAL SOC
- Citation
- ORGANIC LETTERS, v.16, no.14, pp.3720 - 3723
- Indexed
- SCIE
SCOPUS
- Journal Title
- ORGANIC LETTERS
- Volume
- 16
- Number
- 14
- Start Page
- 3720
- End Page
- 3723
- ISSN
- 1523-7060
- Abstract
- An effective metal-free C-H amination of N-Ts-2-alkenylanilines by using DDQ as an oxidant has been developed to afford a diverse range of substituted indoles. This protocol is operationally simple and robust, obviates the need of expensive transition-metal catalysts, and offers a broad substrate scope. A mechanism involving a radical cation generated by SET and a migratorial process via a phenonium ion intermediate is proposed.
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Related Researcher
- Youn, So Won
- COLLEGE OF NATURAL SCIENCES (DEPARTMENT OF CHEMISTRY)