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Technical benefits of using methane as a pyrolysis medium for catalytic pyrolysis of Kraft lignin

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dc.contributor.authorFarooq, Abid-
dc.contributor.authorShiung Lam, Su-
dc.contributor.authorHoon Rhee, Gwang-
dc.contributor.authorLee, Jechan-
dc.contributor.authorAli Khan, Moonis-
dc.contributor.authorJeon, Byong-Hun-
dc.contributor.authorPark, Young-Kwon-
dc.date.accessioned2022-07-19T05:01:14Z-
dc.date.available2022-07-19T05:01:14Z-
dc.date.created2022-05-04-
dc.date.issued2022-06-
dc.identifier.issn0960-8524-
dc.identifier.urihttps://scholarworks.bwise.kr/hanyang/handle/2021.sw.hanyang/170132-
dc.description.abstractCatalytic fast pyrolysis of low sulfonated Kraft lignin was performed under different atmospheric environments such as N2, CH4, and the gas derived from CH4 decomposition (CH4-D). The use of Zn- or Mo-loaded HZSM-5 as catalyst led to a higher pyrolytic oil yield compared to parent HZSM-5 in CH4 and CH4-D atmospheres. The yields of benzene, toluene, and xylenes were increased by the synergistic effects from metal loading, higher H/Ceff ratio, higher acidity, and CH4 activation. The enhanced CH4 activation via metal loading resulted in higher methylation of alkyl moieties and 33% increase in the total yield of benzene, toluene, and xylenes in comparison to parent HZSM-5. A higher H/Ceff ratio of 6 via CH4 decomposition led to the formation of a hydro-pyrolysis environment. Moreover, the CH4-D environment showed H2/CH4 ratio of 0.36 in the product gas which warranted the presence of more H2 under the CH4-D pyrolysis environment.-
dc.language영어-
dc.language.isoen-
dc.publisherElsevier Ltd-
dc.titleTechnical benefits of using methane as a pyrolysis medium for catalytic pyrolysis of Kraft lignin-
dc.typeArticle-
dc.contributor.affiliatedAuthorJeon, Byong-Hun-
dc.identifier.doi10.1016/j.biortech.2022.127131-
dc.identifier.scopusid2-s2.0-85128178863-
dc.identifier.wosid000795623000001-
dc.identifier.bibliographicCitationBioresource Technology, v.353, pp.1 - 6-
dc.relation.isPartOfBioresource Technology-
dc.citation.titleBioresource Technology-
dc.citation.volume353-
dc.citation.startPage1-
dc.citation.endPage6-
dc.type.rimsART-
dc.type.docTypeArticle-
dc.description.journalClass1-
dc.description.isOpenAccessN-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.relation.journalResearchAreaAgriculture-
dc.relation.journalResearchAreaBiotechnology & Applied Microbiology-
dc.relation.journalResearchAreaEnergy & Fuels-
dc.relation.journalWebOfScienceCategoryAgricultural Engineering-
dc.relation.journalWebOfScienceCategoryBiotechnology & Applied Microbiology-
dc.relation.journalWebOfScienceCategoryEnergy & Fuels-
dc.subject.keywordPlusAROMATIC-HYDROCARBONS-
dc.subject.keywordPlusCONVERSION-
dc.subject.keywordPlusBIOFUELS-
dc.subject.keywordPlusBIOMASS-
dc.subject.keywordPlusZN-
dc.subject.keywordAuthorMethane decomposition-
dc.subject.keywordAuthorAromatics-
dc.subject.keywordAuthorZeolites-
dc.subject.keywordAuthorKraft Lignin-
dc.identifier.urlhttps://www.sciencedirect.com/science/article/pii/S0960852422004606?via%3Dihub-
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