H2 generation from steam gasification of swine manure over nickel-loaded perovskite oxides catalysts
DC Field | Value | Language |
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dc.contributor.author | Valizadeh, Soheil | - |
dc.contributor.author | Khani, Yasin | - |
dc.contributor.author | Yim, Hoesuk | - |
dc.contributor.author | Chai, Suhyeong | - |
dc.contributor.author | Chang, Dongwon | - |
dc.contributor.author | Farooq, Abid | - |
dc.contributor.author | Show, Pau-Loke | - |
dc.contributor.author | Jeon, Byong-Hun | - |
dc.contributor.author | Khan, Moonis Ali | - |
dc.contributor.author | Jung, Sang-Chul | - |
dc.contributor.author | Park, Young-Kwon | - |
dc.date.accessioned | 2023-05-03T11:09:30Z | - |
dc.date.available | 2023-05-03T11:09:30Z | - |
dc.date.created | 2023-01-05 | - |
dc.date.issued | 2023-02 | - |
dc.identifier.issn | 0013-9351 | - |
dc.identifier.uri | https://scholarworks.bwise.kr/hanyang/handle/2021.sw.hanyang/185160 | - |
dc.description.abstract | In this study, nickel-loaded perovskite oxides catalysts were synthesized via the impregnation of 10%Ni on XTiO3 (X = Ce, Sr, La, Ba, Ca, and Fe) supports and employed in the catalytic steam gasification of swine manure to produce H2-rich syngas for the first time. The synthesized catalysts were characterized using BET, H2-TPR, XRD, HR-TEM, and EDX analysis. Briefly, using perovskite supports resulted in the production of ultrafine catalyst nanoparticles with a uniform dispersion of Ni particles. According to the catalytic activity test, the gas yield showed the increment as 10% Ni/LaTiO3 < 10% Ni/FeTiO3 < 10% Ni/CeTiO3 < 10% Ni/BaTiO3 < 10% Ni/SrTiO3 < 10% Ni/CaTiO3. Meanwhile, zero coke formation was achieved due to the oxygen mobility of prepared catalysts. Also, the increase in the H2 production for the applied catalysts was in the sequence as 10% Ni/CeTiO3 < 10% Ni/FeTiO3 < 10% Ni/LaTiO3 < 10% Ni/BaTiO3 < 10% Ni/SrTiO3 < 10% Ni/CaTiO3. The maximum H2 selectivity (∼48 vol%) obtained by10% Ni/CaTiO3 was probably due to the synergistic effect of Ni and Ti on enhancing the water-gas shift reaction, and Ca on creating the maximum oxygen mobility compared to other alkaline earth metals doped at the A place of perovskite. Overall, this study provides a suitable solution for enhanced H2 production through steam gasification of swine manure along with suggesting the appropriate supports to prevent Ni deactivation by lowering coke formation at the same time. | - |
dc.language | 영어 | - |
dc.language.iso | en | - |
dc.publisher | ACADEMIC PRESS INC ELSEVIER SCIENCE | - |
dc.title | H2 generation from steam gasification of swine manure over nickel-loaded perovskite oxides catalysts | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Jeon, Byong-Hun | - |
dc.identifier.doi | 10.1016/j.envres.2022.115070 | - |
dc.identifier.scopusid | 2-s2.0-85144424479 | - |
dc.identifier.wosid | 000950863900001 | - |
dc.identifier.bibliographicCitation | ENVIRONMENTAL RESEARCH, v.219, pp.1 - 9 | - |
dc.relation.isPartOf | ENVIRONMENTAL RESEARCH | - |
dc.citation.title | ENVIRONMENTAL RESEARCH | - |
dc.citation.volume | 219 | - |
dc.citation.startPage | 1 | - |
dc.citation.endPage | 9 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.isOpenAccess | N | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Environmental Sciences & Ecology | - |
dc.relation.journalResearchArea | Public, Environmental & Occupational Health | - |
dc.relation.journalWebOfScienceCategory | Environmental Sciences | - |
dc.relation.journalWebOfScienceCategory | Public, Environmental & Occupational Health | - |
dc.subject.keywordPlus | SUPERCRITICAL WATER GASIFICATION | - |
dc.subject.keywordPlus | HYDROGEN-PRODUCTION | - |
dc.subject.keywordPlus | OXYGEN VACANCIES | - |
dc.subject.keywordPlus | METHANE | - |
dc.subject.keywordPlus | CO2 | - |
dc.subject.keywordPlus | GAS | - |
dc.subject.keywordPlus | PRETREATMENT | - |
dc.subject.keywordPlus | MICROALGAE | - |
dc.subject.keywordPlus | ENERGY | - |
dc.subject.keywordAuthor | Cow manure | - |
dc.subject.keywordAuthor | Catalytic gasification | - |
dc.subject.keywordAuthor | Ni loaded perovskite | - |
dc.subject.keywordAuthor | Hydrogen | - |
dc.subject.keywordAuthor | Coke | - |
dc.identifier.url | https://www.sciencedirect.com/science/article/pii/S0013935122023970?via%3Dihub | - |
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