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A Regio- and Diastereoselective Stille Coupling/Intramolecular Diels-Alder Cascade for the Generation of Fused Pyridines and Application in the Synthesis of (+)-Lycopladine A and (-)-Lycoposerramine R
- Authors
- Sim, Kyu-Hyun; ul Ansari, Thameem; Park, Yong-Gyu; Jeong, Yeolib; Oh, Sang-Ha; Min, Hye-Won; Jeon, Da-Yoon; Kim, Hyunwoo; Cho, Cheon-Gyu
- Issue Date
- Sep-2022
- Publisher
- WILEY-V C H VERLAG GMBH
- Keywords
- Cascade Reactions; Cycloaddition; Diels-Alder Reaction; Stille Cross-Coupling; Total Synthesis
- Citation
- ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.61, no.42, pp.1 - 5
- Indexed
- SCIE
SCOPUS
- Journal Title
- ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
- Volume
- 61
- Number
- 42
- Start Page
- 1
- End Page
- 5
- ISSN
- 1433-7851
- Abstract
- 2-Pyrones with a chiral branched allylic silyl ether substituent underwent intramolecular Diels-Alder reactions with remarkably high pi-facial- and endo-selectivities. The resulting diastereomerically and enantiomerically pure cycloadducts were transformed into the natural products (+)-lycopladine A and (-)-lycoposerramine R.
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Related Researcher
- Cho, Cheon Gyu
- COLLEGE OF NATURAL SCIENCES (DEPARTMENT OF CHEMISTRY)