A General Strategy of Anion-Rich High-Concentration Polymeric Interlayer for High-Voltage, All-Solid-State Batteries
DC Field | Value | Language |
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dc.contributor.author | Bae, Jiwoong | - |
dc.contributor.author | Zhang, Xiao | - |
dc.contributor.author | Guo, Xuelin | - |
dc.contributor.author | Yu, Guihua | - |
dc.date.accessioned | 2023-08-16T08:00:15Z | - |
dc.date.available | 2023-08-16T08:00:15Z | - |
dc.date.issued | 2021-01 | - |
dc.identifier.issn | 1530-6984 | - |
dc.identifier.issn | 1530-6992 | - |
dc.identifier.uri | https://scholarworks.bwise.kr/hanyang/handle/2021.sw.hanyang/189226 | - |
dc.description.abstract | All-solid-state batteries are promising energy storage systems as a power source for future electric applications. However, the solid electrolytes have suffered from oxidative vulnerability at the catalytic cathode's surface, particularly at the high-voltage charging process. The poor charge transport and the contact issue at the electrolyte/electrode interface also hamper fully utilizing high-energy-density batteries. In this work, a general design of a high-concentration polymeric interlayer is developed. The interactions between a number of anions in the high-salt-concentration and the polymer chain's functional groups have shown outstanding physicochemical properties, including the rich solvation sites and conductive nanochannels, which Li+ ions can coordinate to or conduct through. The high-concentration polymeric interlayer is also highly resistant to oxidation (up to 5 V) that leads to significant improvement in cycle life with various cathodes, including LiNi1/3Co1/3Mn1/3O2, LiCoO2 and LiFePO4, demonstrating a high Coulombic efficiency over 99.9%. | - |
dc.format.extent | 8 | - |
dc.language | 영어 | - |
dc.language.iso | ENG | - |
dc.publisher | AMER CHEMICAL SOC | - |
dc.title | A General Strategy of Anion-Rich High-Concentration Polymeric Interlayer for High-Voltage, All-Solid-State Batteries | - |
dc.type | Article | - |
dc.publisher.location | 미국 | - |
dc.identifier.doi | 10.1021/acs.nanolett.0c04959 | - |
dc.identifier.scopusid | 2-s2.0-85100120887 | - |
dc.identifier.wosid | 000614066800041 | - |
dc.identifier.bibliographicCitation | NANO LETTERS, v.21, no.2, pp 1184 - 1191 | - |
dc.citation.title | NANO LETTERS | - |
dc.citation.volume | 21 | - |
dc.citation.number | 2 | - |
dc.citation.startPage | 1184 | - |
dc.citation.endPage | 1191 | - |
dc.type.docType | 정기 학술지(letter(letters to the editor)) | - |
dc.description.isOpenAccess | N | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.relation.journalResearchArea | Science & Technology - Other Topics | - |
dc.relation.journalResearchArea | Materials Science | - |
dc.relation.journalResearchArea | Physics | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Physical | - |
dc.relation.journalWebOfScienceCategory | Nanoscience & Nanotechnology | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.relation.journalWebOfScienceCategory | Physics, Applied | - |
dc.relation.journalWebOfScienceCategory | Physics, Condensed Matter | - |
dc.subject.keywordAuthor | solid-state battery | - |
dc.subject.keywordAuthor | high concentration | - |
dc.subject.keywordAuthor | lithium-ion conductor | - |
dc.subject.keywordAuthor | polymer coating | - |
dc.subject.keywordAuthor | high-voltage cathode | - |
dc.identifier.url | https://pubs.acs.org/doi/10.1021/acs.nanolett.0c04959 | - |
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