All-in-One Synthesis of Mesoporous Silicon Nanosheets from Natural Clay and Their Applicability in Hydrogen Evolution
DC Field | Value | Language |
---|---|---|
dc.contributor.author | Ryu, Jaegeon | - |
dc.contributor.author | Jang, Youn Jeong | - |
dc.contributor.author | Choi, Sinho | - |
dc.contributor.author | Kang, Hyun Joon | - |
dc.contributor.author | Park, Hyungmin | - |
dc.contributor.author | Lee, Jae Sung | - |
dc.contributor.author | Park, Soojin | - |
dc.date.accessioned | 2021-08-02T17:26:51Z | - |
dc.date.available | 2021-08-02T17:26:51Z | - |
dc.date.created | 2021-05-14 | - |
dc.date.issued | 2016-03 | - |
dc.identifier.issn | 1884-4049 | - |
dc.identifier.uri | https://scholarworks.bwise.kr/hanyang/handle/2021.sw.hanyang/23868 | - |
dc.description.abstract | Silicon nanosheets have attracted much attention owing to their novel electronic and optical properties and compatibility with existing silicon technology. However, a cost-effective and scalable technique for synthesizing these nanosheets remains elusive. Here, we report a novel strategy for producing silicon nanosheets on a large scale through the simultaneous molten-salt-induced exfoliation and chemical reduction of natural clay. The silicon nanosheets thus synthesized have a high surface area, are ultrathin (similar to 5 nm) and contain mesoporous structures derived from the oxygen vacancies in the clay. These advantages make the nanosheets a highly suitable photocatalyst with an exceptionally high activity for the generation of hydrogen from a water-methanol mixture. Further, when the silicon nanosheets are combined with platinum as a cocatalyst, they exhibit high activity in KOH (15.83 mmol H-2 per s per mol Si) and excellent photocatalytic activity with respect to the evolution of hydrogen from a water-methanol mixture (723 mu mol H-2 per h per g Si). | - |
dc.language | 영어 | - |
dc.language.iso | en | - |
dc.publisher | NATURE PUBLISHING GROUP | - |
dc.title | All-in-One Synthesis of Mesoporous Silicon Nanosheets from Natural Clay and Their Applicability in Hydrogen Evolution | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Jang, Youn Jeong | - |
dc.identifier.doi | 10.1038/am.2016.35 | - |
dc.identifier.scopusid | 2-s2.0-84979598447 | - |
dc.identifier.wosid | 000373890300006 | - |
dc.identifier.bibliographicCitation | NPG ASIA MATERIALS, v.8, pp.1 - 9 | - |
dc.relation.isPartOf | NPG ASIA MATERIALS | - |
dc.citation.title | NPG ASIA MATERIALS | - |
dc.citation.volume | 8 | - |
dc.citation.startPage | 1 | - |
dc.citation.endPage | 9 | - |
dc.type.rims | ART | - |
dc.type.docType | 정기학술지(Article(Perspective Article포함)) | - |
dc.description.journalClass | 1 | - |
dc.description.isOpenAccess | Y | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Materials Science | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.subject.keywordPlus | SURFACE-AREA | - |
dc.subject.keywordPlus | BAND-GAP | - |
dc.subject.keywordPlus | WATER | - |
dc.subject.keywordPlus | LIGHT | - |
dc.subject.keywordPlus | ANODES | - |
dc.subject.keywordPlus | HEAT | - |
dc.subject.keywordPlus | SI | - |
dc.identifier.url | https://www.nature.com/articles/am201635 | - |
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