Multiwalled Carbon Nanotubes Anode in Lithium-Ion Battery with LiCoO2, Li[Ni1/3Co1/3Mn1/3]O2, and LiFe1/4Mn1/2Co1/4PO4 Cathodes
- Authors
- Di Lecce, Daniele; Andreotti, Paolo; Boni, Mattia; Gasparro, Giulia; Rizzati, Giulia; Hwang, Jang-Yeon; Sun, Yang-Kook; Hassoun, Jusef
- Issue Date
- Mar-2018
- Publisher
- AMER CHEMICAL SOC
- Keywords
- Multiwalled carbon nanotubes; LiCoO2; Li[Ni1/3Co1/3Mn1/3]O-2; LiFe1/4Mn1/2Co1/4PO4; Li-ion battery
- Citation
- ACS SUSTAINABLE CHEMISTRY & ENGINEERING, v.6, no.3, pp.3225 - 3232
- Indexed
- SCIE
SCOPUS
- Journal Title
- ACS SUSTAINABLE CHEMISTRY & ENGINEERING
- Volume
- 6
- Number
- 3
- Start Page
- 3225
- End Page
- 3232
- URI
- https://scholarworks.bwise.kr/hanyang/handle/2021.sw.hanyang/4726
- DOI
- 10.1021/acssuschemeng.7b03395
- ISSN
- 2168-0485
- Abstract
- Multiwalled carbon nanotubes (MWCNTs) are studied for the first time as the anode in lithium-ion batteries using LiCoO2, Li[Ni1/3Co1/3Mn1/3]O2, and LiFe1/4Mn1/2Co1/4PO4 cathodes. The anode material has a partially graphitic structure and nanotube morphology, which ensure stable cycling, Coulombic efficiency exceeding 99% as well as remarkable rate-capability in lithium half-cell, and suggest the compatibility for full-cell application. The performance of each lithium-ion array appears strongly related to the different structural, morphological and electrochemical features of the positive electrodes. The study in full-cell of the MWCNTs anode, to date mostly investigated in lithium half-cell, is therefore performed under various conditions. The MWCNTs/Li[Ni1/3Co1/3Mn1/3]O2 combination reveals promising behavior in terms of cycling stability, reversible capacity and Coulombic efficiency, which well demonstrates the potential suitability of MWCNTs as anodes in lithium-ion cell.
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