Removal of selected pharmaceuticals and personal care products in reclaimed water during simulated managed aquifer recharge

Abstract

This study investigated the removal of selected pharmaceuticals and personal care products (PPCPs) in a simulated managed aquifer recharge (MAR) system. The PPCPs included antibiotic, antiepileptic, antihypertensive, anti-inflammatory, and antilipidemic drugs, contrast media, herbicides, and stimulants. We first monitored the occurrence and fate of 22 PPCPs at a water reclamation facility (WRF) in Korea, and found carbamazepine and primidone were not readily removed (below 25% removal in average) by the WRF. This reclaimed water passed through a laboratory-scale soil column set-up at 0.5 m/d over one year, simulating MAR system. Atenolol, propranolol, and trimethoprim exhibited higher removal rates (> 80%) than other PPCPs through the simulated MAR, while atrazine, carbamazepine, lincomycin, primidone, and sulfamethazine were not readily removed, exhibiting removal rates below 20%. It can be efficient to monitor and manage these recalcitrant compounds at MAR systems to improve water quality. (C) 2018 Elsevier B.V. All rights reserved.