Phonon anomalies and possible local lattice distortions in giant magnetocapacitive CdCr2S4
DC Field | Value | Language |
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dc.contributor.author | Gnezdilov, V. | - |
dc.contributor.author | Lemmens, P. | - |
dc.contributor.author | Pashkevich, Yu G. | - |
dc.contributor.author | Payen, Ch | - |
dc.contributor.author | Choi, K. Y. | - |
dc.contributor.author | Hemberger, J. | - |
dc.contributor.author | Loidl, A. | - |
dc.contributor.author | Tsurkan, V. | - |
dc.date.available | 2019-05-29T11:40:02Z | - |
dc.date.issued | 2011-07 | - |
dc.identifier.issn | 1098-0121 | - |
dc.identifier.issn | 1550-235X | - |
dc.identifier.uri | https://scholarworks.bwise.kr/cau/handle/2019.sw.cau/21408 | - |
dc.description.abstract | We investigate the origin of large magnetocapacitive effects in CdCr2S4 single crystals focusing on phonon anomalies in the fluctuation regime T < T* = 130 K and with the onset of ferromagnetic order T-c = 84.4 K. The observation of longitudinal optical and formerly infrared active modes for T < T-c is used to propose a loss of inversion symmetry and Cr off-centering. Further anomalies in intensity, frequency, and linewidth have an onset temperature T* that coincides with the onset of magnetocapacitive effects. The respective intensity anomalies are attributed in part to an enhanced electronic polarizability of displacements that modulate the Cr-S distance and respective hybridization. This is taken as a prerequisite to the proposed Cr off-centering. Anomalies due to the previously disregarded photodoping and resonance are analyzed comparing different excitation energies. | - |
dc.language | 영어 | - |
dc.language.iso | ENG | - |
dc.publisher | AMER PHYSICAL SOC | - |
dc.title | Phonon anomalies and possible local lattice distortions in giant magnetocapacitive CdCr2S4 | - |
dc.type | Article | - |
dc.identifier.doi | 10.1103/PhysRevB.84.045106 | - |
dc.identifier.bibliographicCitation | PHYSICAL REVIEW B, v.84, no.4 | - |
dc.description.isOpenAccess | N | - |
dc.identifier.wosid | 000292512500003 | - |
dc.identifier.scopusid | 2-s2.0-79961212079 | - |
dc.citation.number | 4 | - |
dc.citation.title | PHYSICAL REVIEW B | - |
dc.citation.volume | 84 | - |
dc.type.docType | Article | - |
dc.publisher.location | 미국 | - |
dc.subject.keywordPlus | MAGNETOELECTRIC MULTIFERROICS | - |
dc.subject.keywordPlus | VIBRATION-SPECTRA | - |
dc.subject.keywordPlus | RAMAN-SCATTERING | - |
dc.subject.keywordPlus | PHASE-TRANSITION | - |
dc.subject.keywordPlus | POLARIZATION | - |
dc.subject.keywordPlus | FERROELECTRICITY | - |
dc.subject.keywordPlus | NANOSTRUCTURES | - |
dc.subject.keywordPlus | PROGRESS | - |
dc.subject.keywordPlus | RELAXOR | - |
dc.subject.keywordPlus | FILMS | - |
dc.relation.journalResearchArea | Materials Science | - |
dc.relation.journalResearchArea | Physics | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.relation.journalWebOfScienceCategory | Physics, Applied | - |
dc.relation.journalWebOfScienceCategory | Physics, Condensed Matter | - |
dc.description.journalRegisteredClass | sci | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
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