Effects of temperature on the nonlinear response function for two-dimensional vibrational spectroscopy
- Authors
- Sung, Jaeyoung; Silbey, Robert J.; Cho, Minhaeng
- Issue Date
- Jul-2001
- Publisher
- AMER INST PHYSICS
- Citation
- JOURNAL OF CHEMICAL PHYSICS, v.115, no.3, pp 1422 - 1428
- Pages
- 7
- Journal Title
- JOURNAL OF CHEMICAL PHYSICS
- Volume
- 115
- Number
- 3
- Start Page
- 1422
- End Page
- 1428
- URI
- https://scholarworks.bwise.kr/cau/handle/2019.sw.cau/55179
- DOI
- 10.1063/1.1379751
- ISSN
- 0021-9606
1089-7690
- Abstract
- We investigate the effects of temperature on the nonlinear response functions associated with various two-dimensional vibrational spectroscopies. It turns out that the system-bath interaction plays an important role in determining the nature of the temperature-dependencies of the nonlinear response functions and spectra of the two-dimensional vibrational spectroscopy. For a model Hamiltonian, we present exact quantum-mechanical expressions for the nonlinear response functions of two-dimensional vibrational spectroscopies in both the time and frequency domains. (C) 2001 American Institute of Physics.
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Collections - College of Natural Sciences > Department of Chemistry > 1. Journal Articles
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