High‐Performance, Flexible NO2 Chemiresistors Achieved by Design of Imine‐Incorporated n‐Type Conjugated Polymers
DC Field | Value | Language |
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dc.contributor.author | Park, Hyeonjung | - |
dc.contributor.author | Kim, Dong-Ha | - |
dc.contributor.author | Ma, Boo Soo | - |
dc.contributor.author | Shin, Euichul | - |
dc.contributor.author | Kim, Youngkwon | - |
dc.contributor.author | Kim, Taek-Soo | - |
dc.contributor.author | Kim, Felix Sunjoo | - |
dc.contributor.author | Kim, Il-Doo | - |
dc.contributor.author | Kim, Bumjoon J. | - |
dc.date.accessioned | 2024-06-11T05:34:00Z | - |
dc.date.available | 2024-06-11T05:34:00Z | - |
dc.date.issued | 2022-05 | - |
dc.identifier.issn | 2198-3844 | - |
dc.identifier.uri | https://scholarworks.bwise.kr/erica/handle/2021.sw.erica/119277 | - |
dc.description.abstract | Flexible and mechanically robust gas sensors are the key technologies for wearable and implantable electronics. Herein, the authors demonstrate the high-performance, flexible nitrogen dioxide (NO2) chemiresistors using a series of n-type conjugated polymers (CPs: PNDIT2/IM-x) and a polymer dopant (poly(ethyleneimine), PEI). Imine double bonds (C = N) are incorporated into the backbones of the CPs with different imine contents (x) to facilitate strong and selective interactions with NO2. The PEI provides doping stability, enhanced electrical conductivity, and flexibility. As a result, the NO2 sensors with PNDIT2/IM-0.1 and PEI (1:1 by weight ratio) exhibit outstanding sensing performances, such as excellent sensitivity (ΔR/Rb = 240% @ 1 ppm), ultralow detection limit (0.1 ppm), high selectivity (ΔR/Rb < 8% @ 1 ppm of interfering analytes), and high stability, thereby outperforming other state-of-the-art CP-based chemiresistors. Furthermore, the thin film of PNDIT2/IM-0.1 and PEI blend is stretchable and mechanically robust, providing excellent flexibility to the NO2 sensors. Our study contributes to the rational design of high-performance flexible gas sensors. © 2022 The Authors. Advanced Science published by Wiley-VCH GmbH. | - |
dc.format.extent | 10 | - |
dc.language | 영어 | - |
dc.language.iso | ENG | - |
dc.publisher | Wiley-VCH Verlag | - |
dc.title | High‐Performance, Flexible NO2 Chemiresistors Achieved by Design of Imine‐Incorporated n‐Type Conjugated Polymers | - |
dc.type | Article | - |
dc.publisher.location | 미국 | - |
dc.identifier.doi | 10.1002/advs.202200270 | - |
dc.identifier.scopusid | 2-s2.0-85126527341 | - |
dc.identifier.wosid | 000770790200001 | - |
dc.identifier.bibliographicCitation | Advanced Science, v.9, no.14, pp 1 - 10 | - |
dc.citation.title | Advanced Science | - |
dc.citation.volume | 9 | - |
dc.citation.number | 14 | - |
dc.citation.startPage | 1 | - |
dc.citation.endPage | 10 | - |
dc.type.docType | 정기학술지(Article(Perspective Article포함)) | - |
dc.description.isOpenAccess | Y | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.relation.journalResearchArea | Science & Technology - Other Topics | - |
dc.relation.journalResearchArea | Materials Science | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary | - |
dc.relation.journalWebOfScienceCategory | Nanoscience & Nanotechnology | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.subject.keywordPlus | GAS-SENSING PROPERTIES | - |
dc.subject.keywordPlus | CONDUCTING POLYMERS | - |
dc.subject.keywordPlus | SIDE-CHAINS | - |
dc.subject.keywordPlus | THIN-FILM | - |
dc.subject.keywordPlus | MECHANICALLY ROBUST | - |
dc.subject.keywordPlus | SENSOR | - |
dc.subject.keywordPlus | CRYSTALLINITY | - |
dc.subject.keywordPlus | TRANSISTORS | - |
dc.subject.keywordPlus | COPOLYMERS | - |
dc.subject.keywordAuthor | conjugated polymer-based chemiresistors | - |
dc.subject.keywordAuthor | flexible sensors | - |
dc.subject.keywordAuthor | high-performance chemiresistors | - |
dc.subject.keywordAuthor | imine bonds | - |
dc.subject.keywordAuthor | NO2 gas sensors | - |
dc.identifier.url | https://onlinelibrary.wiley.com/doi/10.1002/advs.202200270 | - |
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