EXAFS and EPR study of La0.6Sr0.2Ca0.2MnO3 and La0.6Sr0.2Ba0.2MnO3
- Authors
- Yang, Dong-Seok; Ulyanov A.N.; Phan, Manh-Huong; Kim, Ikgyun; Ahn, Byong-Keun; Rhee, Jang Roh; Kim, Jung Sun; Nguyen, Chau; Yu, Seong-Cho
- Issue Date
- Apr-2003
- Publisher
- Elsevier BV
- Keywords
- magnetically ordered materials; spin-lattice interaction; electron paramagnetic resonance; EXAFS
- Citation
- Physica B: Condensed Matter, v.327, no.2-4, pp.183 - 186
- Indexed
- SCIE
SCOPUS
- Journal Title
- Physica B: Condensed Matter
- Volume
- 327
- Number
- 2-4
- Start Page
- 183
- End Page
- 186
- URI
- https://scholarworks.bwise.kr/erica/handle/2021.sw.erica/46700
- DOI
- 10.1016/S0921-4526(02)01722-2
- ISSN
- 0921-4526
- Abstract
- Extended X-ray absorption fine structure (EXAFS) analysis and electron-paramagnetic resonance (EPR) have been used to examine the local structure and the internal dynamics of La0.6Sr0.2Ca0.2MnO3 and La0.6Sr0.2Ba0.2MnO3 lanthanum manganites. The Mn-O bond distance (similar to 1.94Angstrom for both samples) and the Debye-Waller factors (0.36 x 10(-2) and 0.41 X 10(-2) Angstrom(2) for La0.6Sr0.2Ca0.2MnO3 and for La0.6Sr0.2Ba0.2MnO3, respectively) were obtained from the EXAFS analysis. The dependence of the EPR line width on dopant kind (Ca or Ba) showed a decrease of the spin-lattice interaction with an increase of the Curie temperature. For both compositions, the EPR line intensity followed the exponential law I(T) = I-0 exp(E-a/k(B) T), deduced on the basis of the adiabatic polaron hopping model. (C) 2002 Elsevier Science B.V. All rights reserved.
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