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Highly Efficient Phosphorescent Organic Light-Emitting Diodes Using Benzo[4′,5′]imidazo[2′,1′:2,3]imidazo[4,5,1-jk]carbazole as a Rigid and Effective Electron Acceptor in Bipolar Host

Authors
Raikwar, Manish MannulalKim, Seung ChanSun, JinwonChu, ChangwoongLee, Jun Yeob
Issue Date
Aug-2023
Publisher
AMER CHEMICAL SOC
Keywords
bipolar host; phosphorescent device; greendevice; efficiency; efficiency roll-off
Citation
ACS APPLIED MATERIALS & INTERFACES, v.15, no.34, pp 40809 - 40816
Pages
8
Journal Title
ACS APPLIED MATERIALS & INTERFACES
Volume
15
Number
34
Start Page
40809
End Page
40816
URI
https://scholarworks.bwise.kr/gachon/handle/2020.sw.gachon/91808
DOI
10.1021/acsami.3c08099
ISSN
1944-8244
1944-8252
Abstract
A novel bipolar host architecture was investigated toimprove theexternal quantum efficiency (EQE) of green phosphorescent organiclight-emitting diodes (PhOLEDs). The host was developed by incorporatingcarbazole as a hole-transport unit and fused rigid benzo[4 & PRIME;,5 & PRIME;]imidazo[2 & PRIME;,1 & PRIME;:2,3]imidazo[4,5, 1-jk]carbazole (BzICz) as a new electrontransport unit. The primary goal of the BzICz-based hostdesign was to achieve a high triplet energy and bipolar charge transportcharacteristics. The green PhOLEDs fabricated using the new BzICz and carbazole-based host demonstrated a high EQE of26.6% due to their high triplet energy and good bipolar charge transportingcharacteristics.
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Manulal, Raikwar Manish
BioNano Technology (Department of Chemistry)
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