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Infrared study of the electronic structure of the metallic pyrochlore iridate Bi2Ir2O7open access

Authors
Lee, Yun SangMoon, SoonjaeRiggs, Scott C.Shapiro, Maxwell C.Fisher, Ian R.Fulfer, Bradford W.Chan, Julia Y.Kemper, Alexander F.Basov, Dimitri N.
Issue Date
May-2013
Publisher
AMER PHYSICAL SOC
Citation
PHYSICAL REVIEW B, v.87, no.19, pp.1 - 7
Indexed
SCIE
SCOPUS
Journal Title
PHYSICAL REVIEW B
Volume
87
Number
19
Start Page
1
End Page
7
URI
https://scholarworks.bwise.kr/hanyang/handle/2021.sw.hanyang/143737
DOI
10.1103/PhysRevB.87.195143
ISSN
2469-9950
Abstract
We investigated the electronic properties of a single crystal of metallic pyrochlore iridate Bi2Ir2O7 by means of infrared spectroscopy. Our optical conductivity data show the splitting of t(2g) bands into J(eff) ones due to strong spin-orbit coupling. We observed a sizable midinfrared absorption near 0.2 eV which can be attributed to the optical transition within the J(eff, 1/2) bands. More interestingly, we found an abrupt suppression of optical conductivity in the very far-infrared region. Our results suggest that the electronic structure of Bi2Ir2O7 is governed by the strong spin-orbit coupling and correlation effects, which are a prerequisite for theoretically proposed nontrivial topological phases in pyrochlore iridates.
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