Long-Term Stability for Co-Electrolysis of CO2/Steam Assisted by Catalyst-Infiltrated Solid Oxide Cellsopen access
- Authors
- Jeong, Hyeon-Ye; Yoon, Kyung Joong; Lee, Jong-Ho; Chung, Yong-Chae; Hong, Jongsup
- Issue Date
- Jan-2018
- Publisher
- SPRINGER HEIDELBERG
- Keywords
- Solid oxide cells; Catalysts infiltration; Co-electrolysis; CO2 conversion; Long-term stability
- Citation
- JOURNAL OF THE KOREAN CERAMIC SOCIETY, v.55, no.1, pp.50 - 54
- Indexed
- SCOPUS
KCI
- Journal Title
- JOURNAL OF THE KOREAN CERAMIC SOCIETY
- Volume
- 55
- Number
- 1
- Start Page
- 50
- End Page
- 54
- URI
- https://scholarworks.bwise.kr/hanyang/handle/2021.sw.hanyang/17870
- DOI
- 10.4191/kcers.2018.55.1.09
- ISSN
- 1229-7801
- Abstract
- This study investigated the long-term durability of catalyst(Pd or Fe)-infiltrated solid oxide cells for CO2/steam co-electrolysis. Fuel-electrode supported solid oxide cells with dimensions of 5 x 5 cm(2) were fabricated, and palladium or iron was subsequently introduced via wet infiltration (as a form of PdO or FeO solution). The metallic catalysts were employed in the fuel-electrode to promote CO2 reduction via reverse water gas shift reactions. The metal-precursor particles were well-dispersed on the fuel-electrode substrate, which formed a bimetallic alloy with Ni embedded on the substrate during high-temperature reduction processes. These planar cells were tested using a mixture of H2O and CO2 to measure the electrochemical and gas-production stabilities during 350 h of co-electrolysis operations. The results confirmed that compared to the Fe-infiltrated cell, the Pd-infiltrated cell had higher stabilities for both electrochemical reactions and gas-production given its resistance to carbon deposition.
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