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Pivotal Role of Nanoparticle Distribution on Agile Steering of Magnetic Microrobots

Authors
Won, SukyoungKim, MingeunLee, JaeyongKo, Young JoonYang, KijunLee, Hee EunKim, Yong JuJung, Jong HoonKim, Jin KonHyun, KyuWie, Jeong Jae
Issue Date
Jun-2025
Publisher
American Chemical Society
Citation
Chemistry of Materials, v.37, no.12, pp 4350 - 4362
Pages
13
Indexed
SCIE
SCOPUS
Journal Title
Chemistry of Materials
Volume
37
Number
12
Start Page
4350
End Page
4362
URI
https://scholarworks.bwise.kr/hanyang/handle/2021.sw.hanyang/210577
DOI
10.1021/acs.chemmater.5c00290
ISSN
0897-4756
1520-5002
Abstract
Magnetic microrobots can be spatiotemporally steered by manipulating external magnetic fields, achieving rapid locomotion. However, for high-speed magnetic microrobots, steering stability is crucial to control actuation speeds along predetermined trajectories. Herein, we discover that nanoscale distribution of magnetic nanoparticles is key to ensuring the steering stability of agile magnetic microrobots. A model system comprising two different processing methods is implemented to induce either macroscopic phase separation or nanoscale distribution of nanoparticles within thermoplastic nanocomposites-based magnetic microrobots. The dispersive and distributive mixing of magnetic nanoparticles is evaluated via systematic investigation on magnetic, thermal, and rheological properties. According to the spatial distribution states of the magnetic nanoparticles, magnetic microrobots exhibit stark differences in motion uniformity and trajectory regularity during agile pivoting motion. Our findings elucidate the correlations among nanocomposite processing, nanoparticle distribution, physical properties, and magnetic actuation, providing valuable insights for designing stimuli-responsive miniaturized robots with enhanced locomotion control.
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