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Organocatalytic Enantioselective Cycloaddition of o-Quinone Methides with Oxazolones: Asymmetric Synthesis of Dihydrocoumarins
- Authors
- Kim, Kyeong Seop; Jang, Jihoon; Kim, Dae Young
- Issue Date
- 13-Nov-2020
- Publisher
- WILEY-V C H VERLAG GMBH
- Keywords
- Organocatalysis; Cycloaddition; ortho-Quinone methides; Dihydrocoumarins; Oxazolones
- Citation
- ChemistrySelect, v.5, no.42, pp 13259 - 13262
- Pages
- 4
- Journal Title
- ChemistrySelect
- Volume
- 5
- Number
- 42
- Start Page
- 13259
- End Page
- 13262
- ISSN
- 2365-6549
- Abstract
- The organocatalytic enantioselective cycloaddition of ortho-quinone methides with oxazolones promoted by a chiral binaphthyl-modified squaramide bifunctional organocatalyst was developed, allowing an efficient synthesis of chiral dihydrocoumarins with excellent enantioselectivity (up to 97 % ee). This approach represents a practical method for the preparation of chiral 3,4-dihydrocoumarin derivatives.
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Related Researcher
- Kim, Dae Young
- College of Natural Sciences (Department of Chemistry)