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Highly Diastereo- and Enantioselective Organocatalyzed Michael/Oxa-Michael Sequence: Asymmetric Synthesis of Pyranonaphthoquinone Derivatives
- Authors
- Kim, Yong Hwan; Jang, Subin; Kim, Dae Young
- Issue Date
- Oct-2018
- Publisher
- 대한화학회
- Keywords
- 2-Hydroxy-1,4-naphthoquinones; 2-Nitroallylic acetates; Pyranonaphthoquinone; Organocatalysis
- Citation
- Bulletin of the Korean Chemical Society, v.39, no.10, pp 1160 - 1164
- Pages
- 5
- Journal Title
- Bulletin of the Korean Chemical Society
- Volume
- 39
- Number
- 10
- Start Page
- 1160
- End Page
- 1164
- ISSN
- 0253-2964
1229-5949
- Abstract
- An efficient asymmetric synthesis of pyranonaphthoquinones via Michael addition and oxo-Michael cyclization sequence of 2-hydroxy-1,4-naphthoquinone with (E)-2-nitroallylic acetates has been developed. The synthetically useful chiral pyranonaphthoquinone derivatives were obtained in moderate to high yields and high enantioselectivities. This approach offers a facile way to prepare chiral pyranonaphthoquinone derivatives with a wide range of functional group tolerance.
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Related Researcher
- Kim, Dae Young
- College of Natural Sciences (Department of Chemistry)