Perovskite-related (CH3NH3)(3)Sb2Br9 for forming-free memristor and low-energy-consuming neuromorphic computing
- Authors
- Yang, JM[Yang, June-Mo]; Choi, ES[Choi, Eun-Suk]; Kim, SY[Kim, So-Yeon]; Kim, JH[Kim, Jeong-Hoon]; Park, JH[Park, Jin-Hong]; Park, NG[Park, Nam-Gyu]
- Issue Date
- 7-Apr-2019
- Publisher
- ROYAL SOC CHEMISTRY
- Citation
- NANOSCALE, v.11, no.13, pp.6453 - 6461
- Indexed
- SCIE
SCOPUS
- Journal Title
- NANOSCALE
- Volume
- 11
- Number
- 13
- Start Page
- 6453
- End Page
- 6461
- URI
- https://scholarworks.bwise.kr/skku/handle/2021.sw.skku/10182
- DOI
- 10.1039/c8nr09918a
- ISSN
- 2040-3364
- Abstract
- Organic-inorganic halide perovskite materials exhibit excellent memristive properties, such as a high on/off ratio and low switching voltage. However, most studies have focused on Pb-based perovskites. Here, we report on the resistive switching and neuromorphic computing properties of Pb-free perovskite-related MA(3)Sb(2)Br(9) (MA = CH3NH3). The Ag/PMMA/MA(3)Sb(2)Br(9)/ITO devices show forming-free characteristics due to a self-formed conducting filament induced by metallic Sb present in the as-prepared MA(3)Sb(2)Br(9) layer. An MA(3)Sb(2)Br(9)-based memristor exhibits a reliable on/off ratio (approximate to 10(2)), an endurance of 300 cycles, a retention time of approximate to 10(4) s and multilevel storage characteristics. Furthermore, synaptic characteristics, such as short-term potentiation, short-term depression and long-term potentiation, are revealed along with a low energy-consumption of 117.9 fJ m(-2), which indicates that MA(3)Sb(2)Br(9) is a promising material for neuromorphic computing.
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