Enhanced thermal stability of Ni nanoparticles in ordered mesoporous supports for dry reforming of methane with CO2
- Authors
- Park, K.S.[Park, K.S.]; Cho, J.M.[Cho, J.M.]; Park, Y.M.[Park, Y.M.]; Kwon, J.H.[Kwon, J.H.]; Yu, J.S.[Yu, J.S.]; Jeong, H.E.[Jeong, H.E.]; Choung, J.W.[Choung, J.W.]; Bae, J.W.[Bae, J.W.]
- Issue Date
- 1-Apr-2022
- Publisher
- Elsevier B.V.
- Keywords
- Dry reforming of methane with CO2 (DRM); Ninanoparticles (NPs); Ordered mesoporous SBA-15; Resistance to aggregation; Spatial confinement effect
- Citation
- Catalysis Today, v.388, pp.224 - 230
- Indexed
- SCIE
SCOPUS
- Journal Title
- Catalysis Today
- Volume
- 388
- Start Page
- 224
- End Page
- 230
- URI
- https://scholarworks.bwise.kr/skku/handle/2021.sw.skku/6998
- DOI
- 10.1016/j.cattod.2020.07.016
- ISSN
- 0920-5861
- Abstract
- Simple strategy to stably preserve the smaller Ni nanoparticles (NPs) having homogeneous crystallite size of ∼5 nm was proposed using ordered mesoporous supports under dry reforming of methane with CO2 (DRM). The NPs-impregnated ordered mesoporous SBA-15 was effective to preserve the smaller Ni nanoparticles with their lower thermal aggregations and less coke depositions by their spatial confinement effects inside of the ordered mesopore structures compared to the irregular conventional SiO2 support. Although the highly ordered mesoporous NPs-impregnated Al2O3 was also found to be effective, the acidic natures of the Al2O3 surfaces accelerated coke depositions by preferentially forming inactive phases. © 2020 Elsevier B.V.
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Collections - Engineering > Chemical Engineering > 1. Journal Articles
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