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Orbital-driven electronic structure changes and the resulting optical anisotropy of the quasi-two-dimensional spin gap compound La4Ru2O10

Authors
Moon, S. J.Choi, W. S.Kim, S. J.Lee, Y. S.Khalifah, P. G.Mandrus, D.Noh, T. W.
Issue Date
21-Mar-2008
Publisher
AMER PHYSICAL SOC
Citation
PHYSICAL REVIEW LETTERS, v.100, no.11
Journal Title
PHYSICAL REVIEW LETTERS
Volume
100
Number
11
URI
http://scholarworks.bwise.kr/ssu/handle/2018.sw.ssu/16891
DOI
10.1103/PhysRevLett.100.116404
ISSN
0031-9007
Abstract
We investigated the electronic response of the quasi-two-dimensional spin gap compound La4Ru2O10 using optical spectroscopy. We observed the drastic changes in the optical spectra as the temperature decreased, resulting in anisotropy in the electronic structure of the spin-singlet ground state. Using the orbital-dependent hopping analysis, we found that orbital ordering plays a crucial role in forming the spin gap state in the non-one-dimensional material.
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