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Dehydrogenation of formic acid using molecular Rh and Ir catalysts immobilized on bipyridine-based covalent triazine frameworks
- Issue Date
- Apr-2019
- Publisher
- ROYAL SOC CHEMISTRY
- Citation
- SUSTAINABLE ENERGY & FUELS, v.3, no.4, pp 1042 - 1047
- Pages
- 6
- Journal Title
- SUSTAINABLE ENERGY & FUELS
- Volume
- 3
- Number
- 4
- Start Page
- 1042
- End Page
- 1047
- ISSN
- 2398-4902
- Abstract
- In this study, catalytic dehydrogenation of formic acid into H-2/CO2 using half-sandwich Rh(iii)/Ir(iii) catalysts immobilized on variable dimensions of bipyridine-based covalent triazine frameworks (bpy-CTFs) has been described for the first time with a highest initial turnover frequency of 7930 h(-1). A systematic study on the influence of the central metal cation (Rh vs. Ir), CTF architectures and amount of metal loadings on the CTF is presented.
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Collections - College of Natural Sciences > Department of Chemistry > 1. Journal Articles
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