Intrinsic cascading contributions to the fifth- and seventh-order electronically off-resonant Raman spectroscopies
- Authors
- Cho, Minhaeng; Blank, David A.; Sung, Jaeyoung; Park, Kisam; Hahn, Sangjoon; Fleming, Graham R.
- Issue Date
- Feb-2000
- Publisher
- AMER INST PHYSICS
- Citation
- JOURNAL OF CHEMICAL PHYSICS, v.112, no.5, pp 2082 - 2094
- Pages
- 13
- Journal Title
- JOURNAL OF CHEMICAL PHYSICS
- Volume
- 112
- Number
- 5
- Start Page
- 2082
- End Page
- 2094
- URI
- https://scholarworks.bwise.kr/cau/handle/2019.sw.cau/55183
- DOI
- 10.1063/1.480777
- ISSN
- 0021-9606
1089-7690
- Abstract
- The cascading polarization contributing to the femtosecond fifth- and seventh-order coherent Raman scattering processes is obtained in terms of the third- and fifth-order Raman response functions. It is found that four cascading processes contribute to the fifth-order Raman scattering signal. In the case of the seventh-order Raman scattering, there are 34 possible cascading processes contributing to the seventh-order Raman scattering signal, and they are classified as chi((5))x chi((3))- and chi((3))x chi((3))x chi((3))-types depending on the involved low-order nonlinear optical processes. Due to the complicated interference among these polarization fields, it may not be possible to experimentally measure the pure seventh-order Raman scattering signal without contamination from the cascaded contributions. (C) 2000 American Institute of Physics. [S0021-9606(00)00104-5].
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Collections - College of Natural Sciences > Department of Chemistry > 1. Journal Articles
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