Crossover from weak anti-localization to weak localization in inkjet-printed Ti3C2Tx MXene thin-film
DC Field | Value | Language |
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dc.contributor.author | Jin, M.-J. | - |
dc.contributor.author | Um, D.-S. | - |
dc.contributor.author | Ogbeide, O. | - |
dc.contributor.author | Kim, C.-I. | - |
dc.contributor.author | Yoo, J.-W. | - |
dc.contributor.author | Robinson, J.W.A. | - |
dc.date.accessioned | 2024-02-19T05:30:28Z | - |
dc.date.available | 2024-02-19T05:30:28Z | - |
dc.date.issued | 2022-09 | - |
dc.identifier.issn | 2287-237X | - |
dc.identifier.issn | 2287-2388 | - |
dc.identifier.uri | https://scholarworks.bwise.kr/cau/handle/2019.sw.cau/72170 | - |
dc.description.abstract | Two-dimensional (2D) transition metal carbides/nitrides or “MXenes” belong to a diverse-class of layered compounds, which offer composition and electric-field-tunable electrical and physical properties. Although the majority of the MXenes, including Ti3C2Tx, are metallic, they typically show semiconductor-like behaviour in their percolated thin-film structure; this is also the most common structure used for fundamental studies and prototype device development of MXene. Magnetoconductance studies of thin-film MXenes are central to understanding their electronic transport properties and charge carrier dynamics, and also to evaluate their potential for spin-tronics and magnetoelectronics. Since MXenes are produced through solution processing, it is desirable to develop deposition strategies such as inkjet-printing to enable scale-up production with intricate structures/networks. Here, we systematically investigate the extrinsic negative magnetoconductance of inkjet-printed Ti3C2Tx MXene thin-films and report a crossover from weak anti-localization (WAL) to weak localization (WL) near 2.5 K. The crossover from WAL to WL is consistent with strong, extrinsic, spin-orbit coupling, a key property for active control of spin currents in spin-orbitronic devices. From WAL/WL magnetoconductance analysis, we estimate that the printed MXene thin-film has a spin orbit coupling field of up to 0.84 T at 1.9 K. Our results and analyses offer a deeper understanding into microscopic charge carrier transport in Ti3C2Tx, revealing promising properties for printed, flexible, electronic and spin-orbitronic device applications. © 2022 Techno-Press, Ltd. | - |
dc.format.extent | 9 | - |
dc.language | 영어 | - |
dc.language.iso | ENG | - |
dc.publisher | Techno-Press | - |
dc.title | Crossover from weak anti-localization to weak localization in inkjet-printed Ti3C2Tx MXene thin-film | - |
dc.type | Article | - |
dc.identifier.doi | 10.12989/anr.2022.13.3.259 | - |
dc.identifier.bibliographicCitation | Advances in Nano Research, v.13, no.3, pp 259 - 267 | - |
dc.description.isOpenAccess | N | - |
dc.identifier.wosid | 000892381700005 | - |
dc.identifier.scopusid | 2-s2.0-85139309117 | - |
dc.citation.endPage | 267 | - |
dc.citation.number | 3 | - |
dc.citation.startPage | 259 | - |
dc.citation.title | Advances in Nano Research | - |
dc.citation.volume | 13 | - |
dc.type.docType | Article | - |
dc.publisher.location | 대한민국 | - |
dc.subject.keywordAuthor | Inkjet printing | - |
dc.subject.keywordAuthor | Magneto-conductance | - |
dc.subject.keywordAuthor | Mxenes | - |
dc.subject.keywordAuthor | Ti3c2tx network | - |
dc.subject.keywordAuthor | Weak anti-localization (wal) | - |
dc.subject.keywordAuthor | Weak localization (wl) | - |
dc.subject.keywordPlus | TITANIUM CARBIDE MXENE | - |
dc.subject.keywordPlus | ELECTRONIC-PROPERTIES | - |
dc.subject.keywordPlus | MAX PHASE | - |
dc.subject.keywordPlus | TRANSITION | - |
dc.subject.keywordPlus | MAGNETORESISTANCE | - |
dc.subject.keywordPlus | DISPERSIONS | - |
dc.subject.keywordPlus | STABILITY | - |
dc.subject.keywordPlus | METALS | - |
dc.subject.keywordPlus | LAYERS | - |
dc.relation.journalResearchArea | Science & Technology - Other Topics | - |
dc.relation.journalResearchArea | Materials Science | - |
dc.relation.journalWebOfScienceCategory | Nanoscience & Nanotechnology | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
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