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Influence of electron-donating and accepting functionalization of fullerene-based photosensitizers on the charge-generation efficiency of polymer composites

Authors
Choi, JongwanKim, NakjoongOh, Jin-WooSong, HeeseokChoi, MoonhyunHong, JinkeeKim, Felix Sunjoo
Issue Date
Dec-2015
Publisher
KOREAN PHYSICAL SOC
Keywords
Photo-charge generation; Charge-transfer complex; Functionalized fullerene; Photosensitizer; Xerography
Citation
JOURNAL OF THE KOREAN PHYSICAL SOCIETY, v.67, no.11, pp 1998 - 2002
Pages
5
Journal Title
JOURNAL OF THE KOREAN PHYSICAL SOCIETY
Volume
67
Number
11
Start Page
1998
End Page
2002
URI
https://scholarworks.bwise.kr/cau/handle/2019.sw.cau/8852
DOI
10.3938/jkps.67.1998
ISSN
0374-4884
1976-8524
Abstract
We studied a series of fullerene derivatives, which had been functionalized by an electron-donating group (triphenylamine) or an electron-accepting group (cyanobenzene), for use as photosensitizers in photoconducting polymer composites. The functionalized fullerenes were synthesized via the Prato reaction. The electronic energy levels of the fullerene derivatives and photo-charge-generation efficiencies of charge-transfer complex between the photoconducting polymer and the dopant were investigated by using density functional theory calculations, optical absorption spectroscopy, and xerographic discharge methods.
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