The high energy density of pb(Zr1-xTix)O3-pb(Ni1/3Nb2/3)O3 ceramics for piezoelectric energy harvesting devices
- Authors
- Seo, In-Tae; Choi, Chang-Hoi; Kang, In-Young; Nahm, Sahn; Kim, Se Bin; Song, Daniel; Lee, Ju; Sung, Tae Hyun; Paik, Jong-Hoo
- Issue Date
- Dec-2012
- Publisher
- KOREAN ASSOC CRYSTAL GROWTH, INC
- Keywords
- Piezoelectric; Energy harvesting; Sintering; Dielectric constant; Ferroelectric
- Citation
- JOURNAL OF CERAMIC PROCESSING RESEARCH, v.13, no.6, pp.739 - 743
- Indexed
- SCIE
SCOPUS
KCI
- Journal Title
- JOURNAL OF CERAMIC PROCESSING RESEARCH
- Volume
- 13
- Number
- 6
- Start Page
- 739
- End Page
- 743
- URI
- https://scholarworks.bwise.kr/hanyang/handle/2021.sw.hanyang/164106
- ISSN
- 1229-9162
- Abstract
- The energy density of 0.65Pb(Zr1-xTix)-0.35Pb(Ni1/3Nb2/3)O3 [0.65P(Z1-xTx)-0.35PNN] ceramics has been investigated with respect to their structural variations. The 0.65P(Z1-xTx)-0.35PNN ceramic with x = 0.58 exhibited a morphotropic phase boundary (MPB), in which pseudo-cubic and tetragonal structures coexisted. The ε33T/ε0 value of the 0.65P(Z1-xTx)-0.35PNN ceramic decreased considerably on the pseudo-cubic side of the MPB composition, while the d33 slowly decreased on both sides of the MPB. Because the g33 is given by d33/ε33T, the maximum transduction coefficient (d33 × g33) was obtained from the composition on the pseudo-cubic side of the MPB. In particular, the 0.65P(Z0.45T0.55)-0.35PNN (0.65PZT55-0.35PNN) ceramic with a pseudo-cubic structure showed the maximum d33 × g33 value of 16,500 × 10-15 m2/N. Moreover, the 0.65PZT55-0.35PNN ceramics with 1.5 mol% CuO added were well sintered even at 950 °C, and also exhibited a high d33 × g33 value of 15,853 × 10-15 m2/N, indicating that the 0.65PZT55-0.35PNN ceramic with CuO added is a good candidate material for multilayer energy harvesting devices.
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