Role of two-dimensional monolayer MoS2 interlayer in the temperature-dependent longitudinal spin Seebeck effect in Pt/YIG bilayer structures
- Authors
- Park, Chanho; Choi, Jae Won; Park, No-Won; Kim, Gil-Sung; Kikkawa, Takashi; Saitoh, Eiji; Lee, Sang-Kwon
- Issue Date
- Jun-2023
- Publisher
- ROYAL SOC CHEMISTRY
- Citation
- JOURNAL OF MATERIALS CHEMISTRY A, v.11, no.22, pp 11831 - 11839
- Pages
- 9
- Journal Title
- JOURNAL OF MATERIALS CHEMISTRY A
- Volume
- 11
- Number
- 22
- Start Page
- 11831
- End Page
- 11839
- URI
- https://scholarworks.bwise.kr/cau/handle/2019.sw.cau/67252
- DOI
- 10.1039/d3ta01702h
- ISSN
- 2050-7488
2050-7496
- Abstract
- Recently, significant efforts have been invested in improving the spin-voltage by inserting thin ferromagnetic interlayers, including monolayer transition metal dichalcogenide (TMDC) layers, in Pt/Y3Fe5O12 (Pt/YIG) structures at 300 K. However, the temperature dependence of the longitudinal spin Seebeck effect (LSSE) of a Pt/YIG structure with a monolayer (ML) TMDC interlayer and the physics underlying the role of the ML interlayer in the Pt/YIG system remain hitherto unexplored. Herein, we report the temperature-dependent LSSE signals of Pt/YIG bilayer and Pt/ML MoS2/YIG trilayer systems. We observed that the measured inverse spin Hall effect (ISHE) voltages of Pt/ML MoS2/YIG are similar to 27 times lower than that of the Pt/YIG system at 190-300 K. This result can be attributed to both the magnetic selection rule and diamagnetic ML MoS2 interlayer, which plays a critical role in hindering the movement of the spins generated at the interface in the Pt/YIG structure. In addition, we theoretically calculated the temperature dependent ISHE voltages by combining a conventional Boltzmann transport equation with the magnon relaxation time model, and the corresponding results consistent with the experimental results of both the Pt/YIG structures. Our finding represents an important achievement in understanding and measuring the LSSE and provides a promising platform, with a high spin-mixing conductance and thermoelectric performance, for two-dimensional interlayered Pt/YIG systems.
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