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Understanding the Electroluminescence Mechanism of CdSe/ZnS Quantum-Dot Light-Emitting Diodes With a Focus on Charge Carrier Behavior in Quantum-Dot Emissive Layers

Authors
Kim, DongjinLee, SeyoungKim, JimyoungLee, Honyeon
Issue Date
Jun-2023
Publisher
Institute of Electrical and Electronics Engineers
Keywords
Electron traps; Quantum dots; Charge carriers; Light emitting diodes; Voltage; Transient analysis; Performance evaluation; Quantum-dot light-emitting diode; transient electroluminescence; impedance spectroscopy
Citation
IEEE Electron Device Letters, v.44, no.6, pp 959 - 962
Pages
4
Journal Title
IEEE Electron Device Letters
Volume
44
Number
6
Start Page
959
End Page
962
URI
https://scholarworks.bwise.kr/sch/handle/2021.sw.sch/24828
DOI
10.1109/LED.2023.3268078
ISSN
0741-3106
1558-0563
Abstract
We analyzed the electroluminescence (EL) mechanisms of quantum-dotlight-emitting diodes (QLEDs) with a focus on charge carrier trapping/detrapping. Multilayer quantum-dot (QD) emissive layers (EMLs) exhibit low void density and many QD surface traps, which provide high efficiency in the low bias voltage region; the efficiency gradually decreases in the high bias voltage region. The roles played by traps and charge carrier trapping/detrapping during QLED EL were revealed by transient EL and impedance spectroscopy analyses. Charge carrier trapping/detrapping of QLEDs with a multilayer QD EML in the low bias voltage region promoted charge injection, rapid initiation of EL, and high current efficiency. In contrast to the conventional view, traps improved QLED performance.
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